Nanoscopic characterization of light-emitting materials is essential to realize nano-optical devices, which requires nanoscopic spatial resolution far beyond the diffraction limit of light. Cathodoluminescence (CL) is a powerful means to achieve such nano-optical characterization by combining with electron microscopy. However, discrimination between coherent and incoherent CL emissions, when a phosphor material is combined with a resonator, is not trivial. To solve this general problem in such coupled emitter–resonator systems, we take advantage of optical saturation in incoherent CL in the phosphor and propose a method to extract the incoherent component to distinguish the coherent components purely from the resonator. We demonstrate this CL saturation imaging approach using an integrated system of Zn2SiO4 phosphors and a plasmonic resonator array and visualize the resonator-modified luminescence at the nanoscale, which evidence the near-field coupling between the phosphors and the plasmonic resonators.
Hikaru Saito, Yuuichiro Kimura, Kentaro Matsuzaki, Yoshikazu Adachi, Sotatsu Yanagimoto, Kosuke Watanabe, Miki Inada, Takumi Sannomiya
Cathodoluminescence Saturation Imaging to Visualize Emitter-Resonator Coupling
ACS Nano
2025.05.20
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